Optimization of process parameters in coagulation of landfill leachate by Al2(SO4)3 and PACl

Emine Can Güven

doi:10.17776/csj.868426

EN

Optimization of process parameters in coagulation of landfill leachate by Al2(SO4)3 and PACl

Abstract

In this study, landfill leachate treatment by coagulation and optimization of process parameters were aimed. Alum (Al2(SO4)3) and Poly Aluminum Chloride (PACl) were used as coagulants to remove total suspended solids (TSS) from landfill leachate, and coagulant dose, reaction time, and pH were optimized as process variables. The Box-Behnken, one of the response surface methodology designs, was used in modeling the coagulation process. The R2 values were very high (>95%) for TSS removal and the models were sufficiently in good agreement with experimental results. The TSS removal efficiencies in coagulation processes with alum and PACl under optimum process conditions determined by the model were 62.1% and 76.4%, respectively while the experimental values under optimum operating conditions were 60.8% and 75.1% in alum and PACl coagulation processes, respectively. According to the results of the study, both coagulation processes were effective in TSS removal from landfill leachate, and response surface methodology is a useful tool for optimizing the treatment parameters. The removal efficiency of the coagulation process conducted with PACl is higher than that of the alum process. Thus, it can be inferred that PACl is more effective under optimized conditions in this study.

Keywords

References

[1] Luo H., Zeng Y., Cheng Y., He D., Pan X., Recent advances in municipal landfill leachate: A review focusing on its characteristics, treatment and toxicity assessment., Sci. Total Environ., 703 (2020) 135468.
[2] Bakhshoodeh R., Alavi N., Oldham C., Santos R.M., Babaei A.A., Vymazal J., Paydary P., Constructed wetlands for landfill leachate treatment: A review, Ecological Engineering, 146 (2020) 105725.
[3] Hilles A.H., Amr S.S.A., Hussein R.A., Arafa A.I., El-Sebaie O.D., Effect of persulfate and persulfate/H2O2 on biodegradability of an anaerobic stabilized landfill leachate, Waste Manag., 44 (2015) 172-177.
[4] Schiopu A-M., Gavrilescu M., Options for the treatment and management of municipal landfill leachate: common and specific issues, Clean-Soil, Air, Water, 38 (2010) 1101-1110.
[5] Renou S., Givaudan J.G., Poulain S., Dirassouyan F., Moulin P., Landfill leachate treatment: review and opportunity, J Hazard. Mater., 150(3) (2008) 468-493.
[6] Deng Y., Englehardt J.D., Treatment of landfill leachate by the Fenton process, Water Res., 40(20) (2006) 3683-3694.
[7] Goi A., Veressinina Y., Trapido M., Fenton process for landfill leachate treatment: evaluation of biodegradability and toxicity, J Environ. Eng., 136(1) (2010) 46-53.
[8] Akkaya E., Sızıntı sularının havasız çamur yataklı reaktör ve mikrofiltrasyonlu biyoreaktör sistemi ile arıtılabilirliğinin araştırılması, PhD Thesis, Yıldız Tech University, Graduate School of Sciences, 2009.

[9] Bohdziewicz J., Kwarciak A., The application of hybrid system UASB reactor-RO in landfill leachate treatment, Desalination, 222(1-3) (2008) 128-134.
[10] Rui M.L., Daud Z., Latif A.A.A., Coagulation-flocculation in leachate treatment by using ferric chloride and alum as coagulant, Int. J. Eng., 2(4) (2012) 1929-1934.
[11] Maleki A., Zazouli M.A., Izanloo H., Rezaee R. Composting plant leachate treatment by coagulation-flocculation process, Am. J Agric. Environ. Sci., 5(5) (2009) 638-643.
[12] Tatsi A.A., Zouboulis A.I., Matis K.A., Samaras P., Coagulation--flocculation pretreatment of sanitary landfill leachates, Chemosphere, 53(7) (2003) 737-744.
[13] Liu X., Li X.M., Yang Q., Yue X., Shen T.T., Zheng W., Luo K., Sun Y.H, Zeng G.M., Landfill leachate pretreatment by coagulation-flocculation process using iron-based coagulants: Optimization by response surface methodology, Chem Eng. J., 200 (2012) 39-51.
[14] Amor C., De Torres-Socías E., Peres J.A., Maldonado M.I., Oller I., Malato S., Lucas M.S., Mature landfill leachate treatment by coagulation/flocculation combined with Fenton and solar photo-Fenton processes, J Hazard. Mater., 286 (2015) 261-268.
[15] Kaur P., Sangal V.K., Kushwaha J.P., Parametric study of electro-Fenton treatment for real textile wastewater, disposal study and its cost analysis, Int. J Environ. Sci. Technol., 16(2) (2019) 801-810.
[16] Ahmadi M., Rahmani K., Rahmani A., Rahmani H., Removal of benzotriazole by Photo-Fenton like process using nano zero-valent iron: response surface methodology with a Box-Behnken design, Polish J Chem. Technol., 19(1) (2017) 104-112.
[17] Mohadesi M., Shokri A., Treatment of oil refinery wastewater by photo-Fenton process using Box--Behnken design method: kinetic study and energy consumption, Int. J Environ. Sci. Technol., 16(11) (2019) 7349-7356.
[18] APHA, Standard Methods for Examination of Water and Wastewater, 21st ed., American Public Health Association, (2005).
[19] Almomani F., Rahul R.B., Optimizing nutrient removal of moving bed biofilm reactor process using response surface methodology, Bioresource technology, 305 (2020) 123059.
[20] Sultana N., Hossain S.Z., Alam M.S., Hashish M.M.A., Islam M.S., An experimental investigation and modeling approach of response surface methodology coupled with crow search algorithm for optimizing the properties of jute fiber reinforced concrete, Construction and Building Materials, 243 (2020) 118216.
[21] Mohajeri S., Aziz H.A., Isa M.H., Zahed M.A., Adlan M.N., Statistical optimization of process parameters for landfill leachate treatment using electro-Fenton technique, J Hazard. Mater., 176(1-3) (2010) 749-758.
[22] Ciric A., Krajnc B., Heath D., Ogrinc N., Response surface methodology and artificial neural network approach for the optimization of ultrasound-assisted extraction of polyphenols from garlic, Food and Chemical Toxicology, 135 (2020) 110976.
[23] Ahmadi M., Ghanbari F., Madihi-Bidgoli S., Photoperoxi-coagulation using activated carbon fiber cathode as an efficient method for benzotriazole removal from aqueous solutions: Modeling, optimization and mechanism, J. Photochem. Photobiol. A Chem., 322 (2016) 85-94.
[24] Ghafari S., Aziz H.A., Isa M.H., Zinatizadeh A.A., Application of response surface methodology (RSM) to optimize coagulation-flocculation treatment of leachate using poly-aluminum chloride (PAC) and alum, J. Hazard. Mater., 163(2-3) (2009) 650-656.
[25] Zhang H., Ran X., Wu X., Zhang D., Evaluation of electro-oxidation of biologically treated landfill leachate using response surface methodology, J. Hazard. Mater., 188(1-3) (2011) 261-268.
[26] Al-Hamadani Y.A., Yusoff M.S., Umar M., Bashir M.J., Adlan M.N., Application of psyllium husk as coagulant and coagulant aid in semi-aerobic landfill leachate treatment, J. Hazard. Mater., 190(1-3) (2011) 582-587.
[27] Zainol N.A., Aziz H.A., Ibrahim N., Treatment of kulim and kuala sepetang landfills leachates in Malaysia using poly-aluminium chloride (PACl), Res. J. Chem. Sci., 3 (2013) 606X.

Details

Primary Language

English

Subjects

Chemical Engineering

Journal Section

Research Article

Authors

Emine Can Güven ^*
0000-0002-3540-3235
Türkiye

Publication Date

June 30, 2021

Submission Date

January 26, 2021

Acceptance Date

May 20, 2021

Published in Issue

Year 2021 Volume: 42 Number: 2

DOI

https://doi.org/10.17776/csj.868426

IZ

https://izlik.org/JA84GU99KJ

Cite

RIS / Bibtex

APA

Can Güven, E. (2021). Optimization of process parameters in coagulation of landfill leachate by Al2(SO4)3 and PACl. Cumhuriyet Science Journal, 42(2), 493-501. https://doi.org/10.17776/csj.868426

Cited By

Green flocculation for sustainable remediation of municipal landfill leachate using Parkia biglobosa extract: optimization, mechanistic insights and implication for design

Clean Technologies and Environmental Policy

https://doi.org/10.1007/s10098-024-02815-0

Multi-response optimization of coagulation–flocculation process for stabilized landfill leachate treatment using a coagulant based on an industrial effluent

Desalination and Water Treatment

https://doi.org/10.5004/dwt.2022.28388

Öz

Optimization of process parameters in coagulation of landfill leachate by Al2(SO4)3 and PACl

Abstract

Keywords

References

Details

Primary Language

Subjects

Journal Section

Authors

Publication Date

Submission Date

Acceptance Date

Published in Issue

DOI

IZ

Cite

Cited By

Green flocculation for sustainable remediation of municipal landfill leachate using Parkia biglobosa extract: optimization, mechanistic insights and implication for design

Multi-response optimization of coagulation–flocculation process for stabilized landfill leachate treatment using a coagulant based on an industrial effluent