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Engineering Zinc Ion Hybrid Supercapacitor Performance of Graphitic Carbon Nitride Embedded Iron Oxide (Hematite)

Year 2024, , 510 - 518, 30.09.2024

Sevda Yetiman , Fatma Kılıç Dokan , Dilek Aker , Ahmet Özdemir , Mustafa Serdar Onses , Erkan Yılmaz , Ertuğrul Şahmetlioğlu

https://doi.org/10.17776/csj.1234262

Abstract

Zinc-ion hybrid supercapacitors (ZHSC) gain high traction due to the prosperous unification of batteries and supercapacitors. Especially with graphene discovery nano carbonaceous materials have been the most investigated types in energy storage (ES) utilization including ZHSC. Among carbonaceous materials, graphitic carbon nitride (g-C3N4) possessing polymeric layers, quasi graphene arouses extreme interest due to its low-impact structure with economical yet chemical and mechanical stability inflicted by high nitrogen contents. Herein, we aim to examine the g-C3N4 doping effect on the electrochemical performance of hematite (α-Fe2O3) for ZHSC application. The assembled ZHSC device managed to reach the potential window of 2.0 volts with an efficient specific capacitance (Sc) of 280 F g-1 at a current density of 1 A g-1. Moreover, the highest energy and power densities were 38.8 Wh kg-1 and 20 kW kg-1 respectively. With this remarkable efficiency, the α-Fe2O3/g-C3N4 composite material can be considered a promising cathode material for ZHSC

Keywords

Graphitic carbon nitride Iron (III) oxide Zinc-ion hybrid supercapacitor

References

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  • [18] Ji H., Jing X., Xu Y., Yan J., Li H., Li Y., Huang L., Zhang Q., Xu, H., Li, H., Magnetic Gc3n4/Nife2o4 Hybrids With Enhanced Photocatalytic Activity, Rsc Advances, 5 (71) (2015) 57960-57967.
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  • [22] Li J., Chen D., Wu Q., Α‐Fe2o3 Based Carbon Composite As Pure Negative Electrode For Application As Supercapacitor, Eur. J. Inorg. Chem., 2019 (10) (2019) 1301-1312.
  • [23] Song G., Chu Z., Jin W., Sun H., Enhanced Performance Of G-C3n4/Tio2 Photocatalysts For Degradation Of Organic Pollutants Under Visible Light, Chin. J. Chem. Eng, 23(8) (2015) 1326-1334.
  • [24] Jiang H., Ma H., Jin Y., Wang L., Gao F., Lu Q., Hybrid Α-Fe2o3@ Ni (Oh) 2 Nanosheet Composite For High-Rate-Performance Supercapacitor Electrode, Sci. Rep , 6 (1) (2016) 31751.
  • [25] Zheng Y., Zhang X., Zhao J., Yang P., Assembled Fabrication Of Α-Fe2o3/Biocl Heterojunctions With Enhanced Photocatalytic Performance, Appl. Surf. Sci, 430 (2018) 585-594.
  • [26] Nabi G., Riaz K.N., Nazir M., Raza W., Tahir M.B., Rafique M., Malik N., Siddiqa A., Gillani S.S.A., Rizwan M., Cogent Synergic Effect Of Tis2/G-C3n4 Composite With Enhanced Electrochemical Performance For Supercapacitor, Ceram. Int. Ceramics , 46 (17) (2020) 27601-27607.
  • [27] Palanivel B., Hossain M.S., Macadangdang Jr, R.R., Ayappan C., Krishnan V., Marnadu R., Kalaivani T., Alharthi, F.A., Sreedevi G., Activation Of Persulfate For Improved Naproxen Degradation Using Feco2o4@ G-C3n4 Heterojunction Photocatalysts, Acs Omega, 6(50) (2021) 34563-34571.
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  • [29] Kumbul A., Gokturk E., Sahmetlioglu E.,Synthesis, Characterization, Thermal Stability And Electrochemical Properties Of Ortho-Imine-Functionalized Oligophenol Via Enzymatic Oxidative Polycondensation, J. Polym. Res., 23 (2016) 1-11.
  • [30] Turac E., Sahmetlioglu E., Toppare L., Yuruk H., Synthesis, Characterization And Optoelectrochemical Properties Of Poly (2, 5-Di (Thiophen-2-Yl-) 1-(4-(Thiophen-3-Yl) Phenyl)-1h-Pyrrole-Co-Edot), Des. Monomers Polym. , 13(3) (2010) 261-275.
  • [31] Turac E., Sahmetlioglu E., Demircan A., Toppare L., Synthesis And Characterization Of Conducting Copolymer Of Trans‐1‐(4‐Methyl‐3′‐Thienyl)‐2‐(Ferrocenyl) Ethene With Edot, J. Appl. Polym. Sci., 126 (3) (2012) 808-814.
  • [32] Zhu Q., Zhao D., Cheng M., Zhou J., Owusu K.A., Mai L., Yu Y., A New View Of Supercapacitors: Integrated Supercapacitors, Adv. Energy Mater., 9(36) (2019) 1901081.
  • [33] Zhang L., Wu D., Wang G., Xu Y., Li H., Yan X., An Aqueous Zinc-Ion Hybrid Super-Capacitor For Achieving Ultrahigh-Volumetric Energy Density, Chin. J. Chem., 32(2) (2021) 926-931.
  • [34] Sundaresan S., Subramanian D., Raju G., Exploration Of Two Dimensional Moo3-Fe2o3 Nanocomposite For The Fabrication Of High Energy Density Supercapacitor Applications , Inorg. Chem. Commun.,148 (2023) 110360.
  • [35] Mazloum-Ardakani M., Sabaghian F., Yavari M., Ebady A., Sahraie N., Enhance The Performance Of Iron Oxide Nanoparticles In Supercapacitor Applications Through Internal Contact Of Α-Fe2o3@Ceo2 Core-Shell, J. Alloys Compd., 819 (2020) 152949.
  • [36] Geerthana M., Prabhu S., Ramesh R., Hierarchical Α-Fe2o3/Mno2/Rgo Ternary Composites As An Electrode Material For High Performance Supercapacitors Application, J. Energy Storage, 47 (2022) 103529.
  • [37] Guo M., Sun J., Liu Y., Huangfu C., Wang R., Han C., Qu Z., Wang N., Zhao L., Zheng Q., Optimizing Fe2o3-Based Supercapacitor Cathode With Tunable Surface Pseudocapacitance Via Facile In Situ Vulcanization Process, J. Electroanal. Chem., 901 (2021) 115785.
  • [38] Mummoorthi G., Shajahan S., Abu Haija M., Mahalingam U., Rajendran R., Synthesis And Characterization Of Ternary Α-Fe2o3/Nio/Rgo Composite For High-Performance Supercapacitors, Acs Omega, 7(31) (2022) 27390-27399.
  • [39] Zhang S., Yin B., Wang Z., Peter F., Super Long-Life All Solid-State Asymmetric Supercapacitor Based On Nio Nanosheets And Α-Fe2o3 Nanorods, J. Chem. Eng., 306 (2016) 193-203.
  • [40] Liang H., Xia C., Emwas A.-H., Anjum D.H., Miao X., Alshareef H.N., Phosphine Plasma Activation Of Α-Fe2o3 For High Energy Asymmetric Supercapacitors, Nano Energy, 49 (2018) 155-162.

Year 2024, , 510 - 518, 30.09.2024

Sevda Yetiman , Fatma Kılıç Dokan , Dilek Aker , Ahmet Özdemir , Mustafa Serdar Onses , Erkan Yılmaz , Ertuğrul Şahmetlioğlu

https://doi.org/10.17776/csj.1234262

Abstract

References

  • [1] Sharifi S., Rahimi K., Yazdani A., Highly Improved Supercapacitance Properties Of Mnfe2o4 Nanoparticles By Mos2 Nanosheets, Sci. Rep., 11 (1) (2020) 8378.
  • [2] Lazarte J.P.L., Dipasupil R.C., Pasco G.Y.S., Eusebio R.C.P., Orbecido A.H., Doong R.-A., Bautista-Patacsil L., Synthesis Of Reduced Graphene Oxide/Titanium Dioxide Nanotubes (Rgo/Tnt) Composites As An Electrical Double Layer Capacitor, Nanomater, 8(11) (2018) 934.
  • [3] Yetiman S., Pecenek H., Dokan F.K., Onses M.S., Yılmaz E., Sahmetlioglu E., Microwave-Assisted Fabrication Of High-Performance Supercapacitors Based On Electrodes Composed Of Cobalt Oxide Decorated With Reduced Graphene Oxide And Carbon Dot, J. Energy Storage , 49 (2022) 104103.
  • [4] El Ghazaly A., Zheng W., Halim J., Tseng E.N., Persson P.O., Ahmed B., Rosen J., Enhanced Supercapacitive Performance Of Mo1. 33c Mxene Based Asymmetric Supercapacitors In Lithium Chloride Electrolyte, J. Energy Storage, 41 (2021) 203-208.
  • [5] Yetiman S., Karagoz S., Kilic Dokan F., Onses M.S., Yilmaz E., Sahmetlioglu E., Rational Integration Of Zif-8 And Bipo(4) For Energy Storage And Environmental Applications, Acs. Omega, 7(49) (2022) 44878-44891.
  • [6] Şahan H., Ateş M.N., Dokan F.K., Ülgen A., Patat Ş., Synergetic Action Of Doping And Coating On Electrochemical Performance Of Lithium Manganese Spinel As An Electrode Material For Lithium-Ion Batteries, B. Mater Sci. , 38 (2015) 141-149.
  • [7] Mateen, A., Ansari, M.Z., Abbas, Q., Muneeb, A., Hussain, A., Eldin E.T., Alzahrani F.M., Alsaiari N.S., Ali S., Javed M.S., In Situ Nitrogen Functionalization Of 2d-Ti3c2t X-Mxenes For High-Performance Zn-Ion Supercapacitor, Molecules, 27 (21) (2022) 7446.
  • [8] Mateen A., Javed M.S., Khan S., Saleem A., Majeed M.K., Khan A.J., Tahir M.F., Ahmad M.A., Assiri M.A., Peng K.-Q., Metal-Organic Framework-Derived Walnut-Like Hierarchical Co-O-Nanosheets As An Advanced Binder-Free Electrode Material For Flexible Supercapacitor, J. Energy Storage , 49 (2022) 104150.
  • [9] Mateen A., Zubair M., Saleem M., Golubenkova A., Voskressensky L., Alothman A.A., Ouladsmane M., Ahmad A., Javed M.S., A Novel High-Performance Anode Material With An Enlarged Potential Window For A Hybrid Energy Storage System, Energies, 15 (24) (2022) 9577.
  • [10] Hussain S.K., Dudem B., Yu J.S., Enhanced Electrochemical Performance Via Ppy Encapsulated 3d Flower-Like Bismuth Molybdate Nanoplates For High-Performance Supercapacitors , Appl. Surf. Sci. , 478 (2019) 846-856.
  • [11] Yetiman S., Dokan F.K., Onses M.S., Yılmaz E., Sahmetlioglu E., Hybrid Electrodes Composed Of Graphitic Carbon Nitride And Zeolitic Imidazolate Framework‐67 For Supercapacitor Applications, Int. J. Energy Res., 46 (15) (2022) 22730-22743.
  • [12] Kiliç Dokan F., Şahan H., Özdemır B. Özdemır, N. Patat, Ş. Synthesis And Characterization Of Spinel Li4ti5o12 Anode Material By Ctab Assisted Sol-Gel Method, Acta Phys. Pol. A, 125 (2) (2014) 648-649.
  • [13] Şahan H., Dokan F.K., Ülgen A., Patat Ş., Improvement Of Cycling Stability Of Limn2o4 Cathode By Fe2o3 Surface Modification For Li-Ion Battery ,Ionics, 20 (2014) 323-333.
  • [14] Patat S., Rahman S., Dokan F.K., The Effect Of Sodium And Niobium Co-Doping On Electrochemical Performance Of Li4ti5o12 As Anode Material For Lithium-Ion Batteries, Ionics, 28 (7) (2022) 3177-3185.
  • [15] Yetiman S., Dokan F.K., Onses M.S., Huang, X., Yılmaz, E., Sahmetlioglu, E., Asymmetric And Zinc-Ion Hybrid Supercapacitors Based On Iron Oxide And Carbon Dots, J. Energy Storage, 68 (2023) 107608.
  • [16] Abbas Q., Mateen A., Khan A.J., Eldesoky G.E., Idrees A., Ahmad A., Eldin E.T., Das H.T., Sajjad M., Javed M.S., Binder-Free Zinc–Iron Oxide As A High-Performance Negative Electrode Material For Pseudocapacitors, Nanomaterials, 12 (18) (2022) 3154.
  • [17] Liu P., Fan X., Ouyang B., Huang Y., Hao R., Gao S., Liu W., Liu K., A Zn Ion Hybrid Capacitor With Enhanced Energy Density For Anode-Free, J. Power Sources, 518 (2022) 230740.
  • [18] Ji H., Jing X., Xu Y., Yan J., Li H., Li Y., Huang L., Zhang Q., Xu, H., Li, H., Magnetic Gc3n4/Nife2o4 Hybrids With Enhanced Photocatalytic Activity, Rsc Advances, 5 (71) (2015) 57960-57967.
  • [19] Xu M., Han L., Dong S., Facile Fabrication Of Highly Efficient G-C3n4/Ag2o Heterostructured Photocatalysts With Enhanced Visible-Light Photocatalytic Activity, Acs Appl. Mater. Interfaces, 5 (23) (2013) 12533-12540.
  • [20] Zhou S.-X., Tao X.-Y., Ma J., Guo L.-T., Zhu Y.-B., Fan H.-L., Liu, Z.-S., Wei, X.-Y., Synthesis Of Flower-Like Pani/G-C3n4 Nanocomposite As Supercapacitor Electrode, Vacuum, 149 (2018) 175-179.
  • [21] Ragupathi, V., Panigrahi P., Subramaniam N.G., G-C3n4 Doped Mns As High Performance Electrode Material For Supercapacitor Application ,Mater. Lett, 246 (2019) 88-91.
  • [22] Li J., Chen D., Wu Q., Α‐Fe2o3 Based Carbon Composite As Pure Negative Electrode For Application As Supercapacitor, Eur. J. Inorg. Chem., 2019 (10) (2019) 1301-1312.
  • [23] Song G., Chu Z., Jin W., Sun H., Enhanced Performance Of G-C3n4/Tio2 Photocatalysts For Degradation Of Organic Pollutants Under Visible Light, Chin. J. Chem. Eng, 23(8) (2015) 1326-1334.
  • [24] Jiang H., Ma H., Jin Y., Wang L., Gao F., Lu Q., Hybrid Α-Fe2o3@ Ni (Oh) 2 Nanosheet Composite For High-Rate-Performance Supercapacitor Electrode, Sci. Rep , 6 (1) (2016) 31751.
  • [25] Zheng Y., Zhang X., Zhao J., Yang P., Assembled Fabrication Of Α-Fe2o3/Biocl Heterojunctions With Enhanced Photocatalytic Performance, Appl. Surf. Sci, 430 (2018) 585-594.
  • [26] Nabi G., Riaz K.N., Nazir M., Raza W., Tahir M.B., Rafique M., Malik N., Siddiqa A., Gillani S.S.A., Rizwan M., Cogent Synergic Effect Of Tis2/G-C3n4 Composite With Enhanced Electrochemical Performance For Supercapacitor, Ceram. Int. Ceramics , 46 (17) (2020) 27601-27607.
  • [27] Palanivel B., Hossain M.S., Macadangdang Jr, R.R., Ayappan C., Krishnan V., Marnadu R., Kalaivani T., Alharthi, F.A., Sreedevi G., Activation Of Persulfate For Improved Naproxen Degradation Using Feco2o4@ G-C3n4 Heterojunction Photocatalysts, Acs Omega, 6(50) (2021) 34563-34571.
  • [28] Chen X., Kuo D.-H., Lu D., Nanonization Of Gc3n 4 With The Assistance Of Activated Carbon For Improved Visible Light Photocatalysis, Rsc Adv., 6 (71) (2016) 66814-66821.
  • [29] Kumbul A., Gokturk E., Sahmetlioglu E.,Synthesis, Characterization, Thermal Stability And Electrochemical Properties Of Ortho-Imine-Functionalized Oligophenol Via Enzymatic Oxidative Polycondensation, J. Polym. Res., 23 (2016) 1-11.
  • [30] Turac E., Sahmetlioglu E., Toppare L., Yuruk H., Synthesis, Characterization And Optoelectrochemical Properties Of Poly (2, 5-Di (Thiophen-2-Yl-) 1-(4-(Thiophen-3-Yl) Phenyl)-1h-Pyrrole-Co-Edot), Des. Monomers Polym. , 13(3) (2010) 261-275.
  • [31] Turac E., Sahmetlioglu E., Demircan A., Toppare L., Synthesis And Characterization Of Conducting Copolymer Of Trans‐1‐(4‐Methyl‐3′‐Thienyl)‐2‐(Ferrocenyl) Ethene With Edot, J. Appl. Polym. Sci., 126 (3) (2012) 808-814.
  • [32] Zhu Q., Zhao D., Cheng M., Zhou J., Owusu K.A., Mai L., Yu Y., A New View Of Supercapacitors: Integrated Supercapacitors, Adv. Energy Mater., 9(36) (2019) 1901081.
  • [33] Zhang L., Wu D., Wang G., Xu Y., Li H., Yan X., An Aqueous Zinc-Ion Hybrid Super-Capacitor For Achieving Ultrahigh-Volumetric Energy Density, Chin. J. Chem., 32(2) (2021) 926-931.
  • [34] Sundaresan S., Subramanian D., Raju G., Exploration Of Two Dimensional Moo3-Fe2o3 Nanocomposite For The Fabrication Of High Energy Density Supercapacitor Applications , Inorg. Chem. Commun.,148 (2023) 110360.
  • [35] Mazloum-Ardakani M., Sabaghian F., Yavari M., Ebady A., Sahraie N., Enhance The Performance Of Iron Oxide Nanoparticles In Supercapacitor Applications Through Internal Contact Of Α-Fe2o3@Ceo2 Core-Shell, J. Alloys Compd., 819 (2020) 152949.
  • [36] Geerthana M., Prabhu S., Ramesh R., Hierarchical Α-Fe2o3/Mno2/Rgo Ternary Composites As An Electrode Material For High Performance Supercapacitors Application, J. Energy Storage, 47 (2022) 103529.
  • [37] Guo M., Sun J., Liu Y., Huangfu C., Wang R., Han C., Qu Z., Wang N., Zhao L., Zheng Q., Optimizing Fe2o3-Based Supercapacitor Cathode With Tunable Surface Pseudocapacitance Via Facile In Situ Vulcanization Process, J. Electroanal. Chem., 901 (2021) 115785.
  • [38] Mummoorthi G., Shajahan S., Abu Haija M., Mahalingam U., Rajendran R., Synthesis And Characterization Of Ternary Α-Fe2o3/Nio/Rgo Composite For High-Performance Supercapacitors, Acs Omega, 7(31) (2022) 27390-27399.
  • [39] Zhang S., Yin B., Wang Z., Peter F., Super Long-Life All Solid-State Asymmetric Supercapacitor Based On Nio Nanosheets And Α-Fe2o3 Nanorods, J. Chem. Eng., 306 (2016) 193-203.
  • [40] Liang H., Xia C., Emwas A.-H., Anjum D.H., Miao X., Alshareef H.N., Phosphine Plasma Activation Of Α-Fe2o3 For High Energy Asymmetric Supercapacitors, Nano Energy, 49 (2018) 155-162.
There are 40 citations in total.

Details

Primary Language English
Subjects Chemical Engineering
Journal Section Natural Sciences
Authors

Sevda Yetiman 0000-0002-8558-8688

Fatma Kılıç Dokan 0000-0002-5355-2904

Dilek Aker 0000-0003-3407-2750

Ahmet Özdemir 0000-0002-2796-1384

Mustafa Serdar Onses 0000-0001-6898-7700

Erkan Yılmaz 0000-0001-8962-3199

Ertuğrul Şahmetlioğlu 0000-0002-7324-0385

Publication Date September 30, 2024
Submission Date January 16, 2023
Acceptance Date July 5, 2024
Published in Issue Year 2024

Cite

APA Yetiman, S., Kılıç Dokan, F., Aker, D., Özdemir, A., et al. (2024). Engineering Zinc Ion Hybrid Supercapacitor Performance of Graphitic Carbon Nitride Embedded Iron Oxide (Hematite). Cumhuriyet Science Journal, 45(3), 510-518. https://doi.org/10.17776/csj.1234262