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Vehicular and industrial sources of PGEs, Au and Ce in surface soil and roadside soils and dusts from two cities of Turkey

Year 2021, Volume: 25 Issue: 2, 484 - 497, 15.04.2021

Murat Özen Songül Akbulut Özen Uğur Çevik

https://doi.org/10.16984/saufenbilder.765677
Cited By: 2

Abstract

In this study, rhodium, palladium, platinum, gold and cerium were determined by ICP-MS after trace-matrix separation in roadside dusts and soil samples along different motorways in Ankara and Bursa, and in soil samples taken from industrial locations in Nilüfer, Bursa.
The clear presence of Pd and Rh was determined at different traffic locations. Platinum remained below the method’s quantification limit for most of the samples. Results showed that both cities showed relatively high concentrations of; Rh and Pt in tunnels and downtowns, Pd in tunnels, bus stations and crossroads, and Au in downtowns. Consistent with the daily road traffic, relatively high concentrations of Rh, Pd and Pt were determined for Ankara. Based on the limited data available for Pt, Pt:Pd ratios varied between 0.04 and 0.25, and Pt:Rh ratios varied between 0.59 and 2.1.
Measurements at the industrial location showed an average Rh and Pd concentration of 11 and 359 µg/kg, respectively. On the other hand, Au concentrations remained below the method’s quantification limit except for one sampling location. The average Ce concentration was determined as 23 mg/kg. Platinum remained below the method’s quantification limit for all industrial sampling locations.
Overall, high average Rh and Pt concentrations were determined at the traffic sites, while higher average Pd concentration was determined at the industrial locations. Cerium remained consistently below the earth’s crustal levels, which infers that no anthropogenic source can be attributed to Ce.

Keywords

platinum group elements, vehicular traffic industrial region surface soil roadside dusts

References

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Year 2021, Volume: 25 Issue: 2, 484 - 497, 15.04.2021

Murat Özen Songül Akbulut Özen Uğur Çevik

https://doi.org/10.16984/saufenbilder.765677
Cited By: 2

Abstract

References

  • [1] G. Schmidt and H. Palme, “Abundances of Os, Ir, Ru, Rh, Pt and Pd in the Earth’s crust,” in The origin and fractionation of highly siderophile elements in the Earth’s mantle, 1997.
  • [2] F. R. Hartley, Ed., Chemistry of the platinum group metals: recent developments. Amsterdam ; New York: Elsevier, 1991.
  • [3] A. Fornalczyk, “Industrial catalysts as a source of valuable metals,” Journal of Achievements in Materials and Manufacturing Engineering, vol. 55, no. 2, pp. 864–869, Dec. 2012.
  • [4] B. Gómez et al., “Levels and risk assessment for humans and ecosystems of platinum-group elements in the airborne particles and road dust of some European cities,” Sci Total Environ, vol. 299, no. 1–3, pp. 1–19, Nov. 2002, doi: 10.1016/S0048-9697(02)00038-4.
  • [5] C. L. S. Wiseman and F. Zereini, “Airborne particulate matter, platinum group elements and human health: A review of recent evidence,” Science of The Total Environment, vol. 407, no. 8, pp. 2493–2500, Apr. 2009, doi: 10.1016/j.scitotenv.2008.12.057.
  • [6] O. Morton-Bermea, O. Amador-Muñoz, L. Martínez-Trejo, E. Hernández-Álvarez, L. Beramendi-Orosco, and M. E. García-Arreola, “Platinum in PM2.5 of the metropolitan area of Mexico City,” Environ Geochem Health, vol. 36, no. 5, pp. 987–994, Oct. 2014, doi: 10.1007/s10653-014-9613-8.
  • [7] M. Ďuriš, “Geochemical and Ecological Survey of the Prague City Area, Czech Republic,” in Mapping the Chemical Environment of Urban Areas, C. C. Johnson, A. Demetriades, J. Locutura, and R. T. Ottesen, Eds. Chichester, UK: John Wiley & Sons, Ltd, 2011, pp. 364–374.
  • [8] K. Boch and M. Schuster, “Determination of palladium in road dust and sewage sludge ashes,” in Palladium Emissions in the Environment, F. Zereini and F. Alt, Eds. Berlin/Heidelberg: Springer-Verlag, 2006, pp. 191–201.
  • [9] S. J. Parry and K. E. Jarvis, “Temporal and Spatial Variation of Palladium in the Roadside Environment,” in Palladium Emissions in the Environment, F. Zereini and F. Alt, Eds. Berlin/Heidelberg: Springer-Verlag, 2006, pp. 419–432.
  • [10] C. L. S. Wiseman, Z. Hassan Pour, and F. Zereini, “Platinum group element and cerium concentrations in roadside environments in Toronto, Canada,” Chemosphere, vol. 145, pp. 61–67, Feb. 2016, doi: 10.1016/j.chemosphere.2015.11.056.
  • [11] B. Leniewska, B. Godlewskaykiewicz, B. Bocca, S. Caimi, S. Caroli, and A. Hulanicki, “Platinum, palladium and rhodium content in road dust, tunnel dust and common grass in Biaystok area (Poland): a pilot study,” Science of The Total Environment, vol. 321, no. 1–3, pp. 93–104, Apr. 2004, doi: 10.1016/j.scitotenv.2003.07.004.
  • [12] K. H. Ek, G. M. Morrison, and S. Rauch, “Environmental routes for platinum group elements to biological materials—a review,” Science of The Total Environment, vol. 334–335, pp. 21–38, Dec. 2004, doi: 10.1016/j.scitotenv.2004.04.027.
  • [13] K. H. Ek, S. Rauch, G. M. Morrison, and P. Lindberg, “Platinum group elements in raptor eggs, faeces, blood, liver and kidney,” Sci Total Environ, vol. 334–335, pp. 149–159, Dec. 2004, doi: 10.1016/j.scitotenv.2004.04.067.
  • [14] M. T. Jackson, H. M. Prichard, and J. Sampson, “Platinum-group elements in sewage sludge and incinerator ash in the United Kingdom: Assessment of PGE sources and mobility in cities,” Science of The Total Environment, vol. 408, no. 6, pp. 1276–1285, Feb. 2010, doi: 10.1016/j.scitotenv.2009.09.014.
  • [15] I. Bednarova et al., “Study of the influence of platinum, palladium and rhodium on duckweed (Lemna minor),” Neuroendocrinol Lett, vol. 35, no. 2, pp. 35–42, 2014.
  • [16] J. Pawlak, E. Łodyga-Chruścińska, and J. Chrustowicz, “Fate of platinum metals in the environment,” J Trace Elem Med Bio, vol. 28, no. 3, pp. 247–254, Jul. 2014, doi: 10.1016/j.jtemb.2014.03.005.
  • [17] F. Zereini and F. Alt, Eds., Palladium emissions in the environment: analytical methods, environmental assessment and health effects. Berlin ; New York: Springer, 2006.
  • [18] K. E. Jarvis, S. J. Parry, and J. M. Piper, “Temporal and Spatial Studies of Autocatalyst-Derived Platinum, Rhodium, and Palladium and Selected Vehicle-Derived Trace Elements in the Environment,” Environ Sci Technol, vol. 35, no. 6, pp. 1031–1036, Mar. 2001, doi: 10.1021/es0001512.
  • [19] G. Nordberg, Ed., Handbook on the toxicology of metals, 3rd ed. Amsterdam ; Boston: Academic Press, 2007.
  • [20] G. Hutchings, “A golden future,” Nature Chem, vol. 1, no. 7, pp. 584–584, Oct. 2009, doi: 10.1038/nchem.388.
  • [21] J. Kašpar, P. Fornasiero, and N. Hickey, “Automotive catalytic converters: current status and some perspectives,” Catalysis Today, vol. 77, no. 4, pp. 419–449, Jan. 2003, doi: 10.1016/S0920-5861(02)00384-X.
  • [22] F. R. Cassee et al., “Exposure, Health and Ecological Effects Review of Engineered Nanoscale Cerium and Cerium Oxide Associated with its Use as a Fuel Additive,” Critical Reviews in Toxicology, vol. 41, no. 3, pp. 213–229, Mar. 2011, doi: 10.3109/10408444.2010.529105.
  • [23] J. D. Whiteley and F. Murray, “Anthropogenic platinum group element (Pt, Pd and Rh) concentrations in road dusts and roadside soils from Perth, Western Australia,” Science of The Total Environment, vol. 317, no. 1–3, pp. 121–135, Dec. 2003, doi: 10.1016/S0048-9697(03)00359-0.
  • [24] F. Zereini et al., “Concentration and Distribution of Heavy Metals in Urban Airborne Particulate Matter in Frankfurt am Main, Germany,” Environ. Sci. Technol., vol. 39, no. 9, pp. 2983–2989, May 2005, doi: 10.1021/es040040t.
  • [25] V. Lyubomirova, R. Djingova, and J. T. van Elteren, “Fractionation of traffic-emitted Ce, La and Zr in road dusts,” J. Environ. Monit., vol. 13, no. 6, p. 1823, 2011, doi: 10.1039/c1em10187k.
  • [26] S. Akbulut and U. Cevik, “Accumulation of Metals in Roadside Soil, Dust and Pine Needles in Different Characteristic Traffic Areas,” Fresen Environ Bull, vol. 23, no. 2A, pp. 516–522, 2014.
  • [27] A. Ucurum, P. J. Lechler, G. B. Arehart, and F. Molnar, “Platinum-Group Element, Stable Isotope, and Fluid Inclusion Investigation of the Ultramafic Rock-Hosted Gunes-Sogucak Ni-Cu-Sulfide Mineralization in the Gunes Ophiolite, East-Central Turkey,” Int Geol Rev, vol. 49, no. 2, pp. 169–192, Feb. 2007, doi: 10.2747/0020-6814.49.2.169.
  • [28] H. Kozlu, H. Prichard, F. Melcher, P. Fisher, C. Brough, and D. Stueben, “Platinum group element (PGE) mineralisation and chromite geochemistry in the Berit ophiolite (Elbistan/Kahramanmaraş), SE Turkey,” Ore Geol Rev, vol. 60, pp. 97–111, Jul. 2014, doi: 10.1016/j.oregeorev.2013.12.011.
  • [29] M. C. Turhan, “Traffic and Transportation Survey of Highway (KGM), General Directorate of Highways, Turkey,” 2010. [Online]. Available: http://www.kgm.gov.tr/SiteCollectionDocuments/KGMdocuments/Istatistikler/TrafikveUlasimBilgileri/10TrafikUlasimBilgileri%20.pdf.
  • [30] MTA, “General Directorate of Mineral Research and Exploration, Turkey,” 2017. http://yerbilimleri.mta.gov.tr/anasayfa.aspx.
  • [31] N. I. Ward and L. M. Dudding, “Platinum emissions and levels in motorway dust samples: influence of traffic characteristics,” Science of The Total Environment, vol. 334–335, pp. 457–463, Dec. 2004, doi: 10.1016/j.scitotenv.2004.04.049.
  • [32] D. Fliegel, Z. Berner, D. Eckhardt, and D. Stüben, “New data on the mobility of Pt emitted from catalytic converters,” Analytical and Bioanalytical Chemistry, vol. 379, no. 1, pp. 131–136, May 2004, doi: 10.1007/s00216-004-2556-7.
  • [33] J. C. Ely, C. R. Neal, C. F. Kulpa, M. A. Schneegurt, J. A. Seidler, and J. C. Jain, “Implications of Platinum-Group Element Accumulation along U.S. Roads from Catalytic-Converter Attrition,” Environ Sci Technol, vol. 35, no. 19, pp. 3816–3822, Oct. 2001, doi: 10.1021/es001989s.
  • [34] A. N. Riga-Karandinos, C. J. Saitanis, and G. Arapis, “First Study of Anthropogenic Platinum Group Elements in Roadside Top-Soils in Athens, Greece,” Water Air Soil Poll, vol. 172, no. 1–4, pp. 3–20, May 2006, doi: 10.1007/s11270-005-9016-7.
  • [35] J. Fritsche and T. Meisel, “Determination of anthropogenic input of Ru, Rh, Pd, Re, Os, Ir and Pt in soils along Austrian motorways by isotope dilution ICP-MS,” Sci Total Environ, vol. 325, no. 1–3, pp. 145–154, Jun. 2004, doi: 10.1016/j.scitotenv.2003.11.019.
  • [36] L. Qi, M.-F. Zhou, Z. Zhao, J. Hu, and Y. Huang, “The characteristics of automobile catalyst-derived platinum group elements in road dusts and roadside soils: a case study in the Pearl River Delta region, South China,” Environ Earth Sci, vol. 64, no. 6, pp. 1683–1692, Nov. 2011, doi: 10.1007/s12665-010-0635-y.
  • [37] S. Pan, G. Zhang, Y. Sun, and P. Chakraborty, “Accumulating characteristics of platinum group elements (PGE) in urban environments, China,” Sci Total Environ, vol. 407, no. 14, pp. 4248–4252, Jul. 2009, doi: 10.1016/j.scitotenv.2009.03.030.
  • [38] B. Gao, Y. Yu, H. Zhou, and J. Lu, “Accumulation and distribution characteristics of platinum group elements in roadside dusts in Beijing, China,” Environ Toxicol Chem, vol. 31, no. 6, pp. 1231–1238, Jun. 2012, doi: 10.1002/etc.1833.
  • [39] H. Wichmann, G. A. K. Anquandah, C. Schmidt, D. Zachmann, and M. A. Bahadir, “Increase of platinum group element concentrations in soils and airborne dust in an urban area in Germany,” Sci Total Environ, vol. 388, no. 1–3, pp. 121–127, Dec. 2007, doi: 10.1016/j.scitotenv.2007.07.064.
  • [40] M. Sager, H.-T. Chon, and L. Marton, “Spatial variation of contaminant elements of roadside dust samples from Budapest (Hungary) and Seoul (Republic of Korea), including Pt, Pd and Ir,” Environ Geochem Hlth, vol. 37, no. 1, pp. 181–193, Feb. 2015, doi: 10.1007/s10653-014-9639-y.
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There are 46 citations in total.

Details

Primary Language English
Subjects Environmental Sciences, Metrology, Applied and Industrial Physics
Journal Section Research Articles
Authors

Murat Özen 0000-0002-3589-2059

Songül Akbulut Özen 0000-0001-8025-2141

Uğur Çevik 0000-0002-7513-5175

Publication Date April 15, 2021
Submission Date July 7, 2020
Acceptance Date November 17, 2020
Published in Issue Year 2021 Volume: 25 Issue: 2

Cite

APA Özen, M., Akbulut Özen, S., & Çevik, U. (2021). Vehicular and industrial sources of PGEs, Au and Ce in surface soil and roadside soils and dusts from two cities of Turkey. Sakarya University Journal of Science, 25(2), 484-497. https://doi.org/10.16984/saufenbilder.765677
AMA Özen M, Akbulut Özen S, Çevik U. Vehicular and industrial sources of PGEs, Au and Ce in surface soil and roadside soils and dusts from two cities of Turkey. SAUJS. April 2021;25(2):484-497. doi:10.16984/saufenbilder.765677
Chicago Özen, Murat, Songül Akbulut Özen, and Uğur Çevik. “Vehicular and Industrial Sources of PGEs, Au and Ce in Surface Soil and Roadside Soils and Dusts from Two Cities of Turkey”. Sakarya University Journal of Science 25, no. 2 (April 2021): 484-97. https://doi.org/10.16984/saufenbilder.765677.
EndNote Özen M, Akbulut Özen S, Çevik U (April 1, 2021) Vehicular and industrial sources of PGEs, Au and Ce in surface soil and roadside soils and dusts from two cities of Turkey. Sakarya University Journal of Science 25 2 484–497.
IEEE M. Özen, S. Akbulut Özen, and U. Çevik, “Vehicular and industrial sources of PGEs, Au and Ce in surface soil and roadside soils and dusts from two cities of Turkey”, SAUJS, vol. 25, no. 2, pp. 484–497, 2021, doi: 10.16984/saufenbilder.765677.
ISNAD Özen, Murat et al. “Vehicular and Industrial Sources of PGEs, Au and Ce in Surface Soil and Roadside Soils and Dusts from Two Cities of Turkey”. Sakarya University Journal of Science 25/2 (April 2021), 484-497. https://doi.org/10.16984/saufenbilder.765677.
JAMA Özen M, Akbulut Özen S, Çevik U. Vehicular and industrial sources of PGEs, Au and Ce in surface soil and roadside soils and dusts from two cities of Turkey. SAUJS. 2021;25:484–497.
MLA Özen, Murat et al. “Vehicular and Industrial Sources of PGEs, Au and Ce in Surface Soil and Roadside Soils and Dusts from Two Cities of Turkey”. Sakarya University Journal of Science, vol. 25, no. 2, 2021, pp. 484-97, doi:10.16984/saufenbilder.765677.
Vancouver Özen M, Akbulut Özen S, Çevik U. Vehicular and industrial sources of PGEs, Au and Ce in surface soil and roadside soils and dusts from two cities of Turkey. SAUJS. 2021;25(2):484-97.

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